Using the femtosecond Raman-induced polarization spectroscopy (RIPS) technique, we have observed ground vibronic state rotational coherence in gaseous N2, COZ and OZ. Both theoretical and experimental studies are reported. The theory is in excellent agreement with experiment. At earlier pump-probe d
✦ LIBER ✦
Effects of O2–CO2polarization beating on femtosecond coherent anti-Stokes Raman scattering (fs-CARS) spectroscopy of O2
✍ Scribed by W. D. Kulatilaka; J. R. Gord; S. Roy
- Book ID
- 106029889
- Publisher
- Springer
- Year
- 2010
- Tongue
- English
- Weight
- 820 KB
- Volume
- 102
- Category
- Article
- ISSN
- 0721-7269
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## Abstract Coherent anti‐Stokes Raman scattering (CARS) spectroscopy of gas‐phase CO~2~ is demonstrated using a single femtosecond (fs) laser beam. A shaped ultrashort laser pulse with a transform‐limited temporal width of ∼7 fs and spectral bandwidth of ∼225 nm (∼3500 cm^−1^) is employed for simu
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