## Abstract The influence of broadening due to intrinsic molecule and ensemble properties (homogeneous and inhomogeneous broadening) on resonance CARS excitation profiles (CEPs) was investigated by means of a theoretical model. The nonβlinear susceptibility Ο^(3)^ of a homogeneous ensemble of molec
β¦ LIBER β¦
Effect of transfer of excitation on resonance broadening
β Scribed by J. Cooper; D.N. Stacey
- Book ID
- 103768237
- Publisher
- Elsevier Science
- Year
- 1973
- Tongue
- English
- Weight
- 156 KB
- Volume
- 46
- Category
- Article
- ISSN
- 0375-9601
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## Abstract The effect of static inhomogeneous environmental broadening of resonance Raman excitation profiles was investigated. The roles of diagonal and nonβdiagonal terms in the twoβfold sum over the local mode vibrational states in the excited intermediate electronic state are discussed. The th