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Effect of lithium cationization on oxygen atom transfer from the nitro group to the double bond during collision-induced decomposition in certain substituted β-nitrostyrenes

✍ Scribed by K. P. Madhusudanan; L. K. Bajpai; A. P. Bhaduri


Publisher
John Wiley and Sons
Year
1997
Tongue
English
Weight
99 KB
Volume
11
Category
Article
ISSN
0951-4198

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✦ Synopsis


Fast-atom bombardment mass spectra of β-nitrostyrene derivatives give rise to abundant M + • and [M + H] + ions and exhibit a fragmentation pattern attributable to the presence of a nitro group. Collision-induced decomposition (CID) of their [M + H] + ions reveals an additional fragmentation involving oxygen migration to the double bond and leading to the protonated aldehyde. This oxygen migration is the predominant process in the CID of the [M + Li] + adducts which exhibit ions corresponding to the lithiated aldehyde and to elimination of the neutral aldehyde.