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Effect of complexation of silver ion with the glycosyl donor and acceptor on the regio- and stereo-selectivity in the β-mannopyranosylation of 1,3-di-N-benzyloxycarbonyl-2-deoxystreptamine using silver triflate as a promoter in tetrahydrofuran

✍ Scribed by Jun-ichi Tamura; Shigeomi Horito; Juji Yoshimura; Hironobu Hashimoto


Publisher
Elsevier Science
Year
1990
Tongue
English
Weight
973 KB
Volume
207
Category
Article
ISSN
0008-6215

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✦ Synopsis


A pseudodisaccharide, a 5-0-Q?-D-mannopyranosyl)-2-deoxystreptamine derivative, was obtained preferentially when 2,3&tri-O-ally&6-0-benzyl-a-D-mannopyranosyl chloride (1) was used as the glycosyl donor for coupling with I ,3-di-~-~nzyloxyc~bonyl-Z-d~xyst~ptamine

(2) usmg silver t&late as a promoter in tetrahydrofuran. Complexation of the glycosyl acceptor and the ally1 protecting group of the glycosyl donor with the promoter proved important for the regio-and stereo-selective formation of the D-mannopyranosyl linkage.