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Effect of basic set quality and electron correlation on the scale factors of a harmonic force field

✍ Scribed by C. W. Bock; Y. N. Panchenko; V. I. Pupyshev


Publisher
John Wiley and Sons
Year
1990
Tongue
English
Weight
462 KB
Volume
11
Category
Article
ISSN
0192-8651

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✦ Synopsis


The completely optimized structure and harmonic force field of s-trans-buta-l,3-diene are reported at the MP2/6-31G and MP2/6-31G* levels of computation. Sets of empirical scale factors for the calculated force fields are derived and compared with the corresponding values computed at the RHF/4-31G and RHF/6-31G levels. Changes in the scale factors for this series of force fields are discussed. The vibrational frequencies are also reported for thirteen isotopomers of s-trans-buta-l,3-diene using the MP21 6-31G* force field. Some characteristics of the gauche and cis forms of buta-l,&diene are also given.