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Durch Umlagerung induzierte Fragmentierung von 4-Tosyloxymethyl-chinuclidin und vergleichende Solvolyse von 1-Tosyloxymethyl-bicyclo[2,2,2]octan und Neopentyltosylat Fragmentierungsreaktionen, 3. Mitteilung

✍ Scribed by C. A. Grob; R. M. Hoegerle; M. Ohta


Publisher
John Wiley and Sons
Year
1962
Tongue
German
Weight
708 KB
Volume
45
Category
Article
ISSN
0018-019X

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✦ Synopsis


Abstract

A fragmentation reaction can be induced by generating a γ‐amino‐carbonium ion through a Wagner‐Meerwein rearrangement of a δ‐amino‐p‐toluenesulfonic ester. Thus solvolysis of 4‐tosyloxymethyl‐quinuclidine (9a) in aqueous ethanol yields the 4‐methylene‐1‐aza‐cycloheptanes (20a) and (20b).