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Downfield γ-gauche and γ-antiperiplanar effects on 13C NMR chemical shifts exerted by thiophene sulphur

✍ Scribed by J. W. de Haan; M. E. van Dommelen; L. J. M. van de Ven; A. Corvers


Publisher
John Wiley and Sons
Year
1978
Tongue
English
Weight
299 KB
Volume
11
Category
Article
ISSN
0749-1581

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✦ Synopsis


Abstract

The γ‐effects of sulphur on ^13^C NMR chemical shifts have been measured in a series of steroidal compounds containing the thiophene ring in different configurations with respect to the rest of the molecule. The data constitute the first example of downfield effects exerted by sulphur on both gauche and antiperiplanar γ‐carbons. The γ‐gauche effect of sulphur amounts to 1.6–1.8 ppm, the γ‐antiperiplanar effect from practically zero to almost 1 ppm.