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Dissociation of doubly charged SH radicals. An experimental and theoretical study

โœ Scribed by D. Mathur; K. Nagesha; V.R. Marathe

Publisher
Elsevier Science
Year
1992
Tongue
English
Weight
454 KB
Volume
200
Category
Article
ISSN
0009-2614

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โœฆ Synopsis

Ion translational energy spectrometry has been applied to study unimolecular and collision-induced dissociation of dications of the SH radical. Experimentally determined values of the kinetic energy released upon dissociation are satisfactorily correlated with results of high-level ab initio calculations of potential en'eqy curves of the ground and low-lying excited electronic states of SH2+ ions. Quantum-chemical methods in which conf%uration interaction effects are accounted for via the coupled-cluster ap proach are employed.

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## Translational energy spectrometry measurements have been made on Hei ions resulting from 3 keV double-electron capture collisions between He: and Ns. The endoergic energy defect for this reaction is measured to be 43 eV. Potential energy curves have been computed for He: (X Ix+), HeF(Z\*) and