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Displacement of equilibrium in electroenzymatic reactor for acetaldehyde production using yeast alcohol dehydrogenase

✍ Scribed by Robert Lortie; Aziz Fassouane; Jean-Marc Laval; Christian Bourdillon


Publisher
John Wiley and Sons
Year
1992
Tongue
English
Weight
626 KB
Volume
39
Category
Article
ISSN
0006-3592

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✦ Synopsis


Electrochemical regeneration of NAD was performed in a bench scale reactor in which yeast alcohol dehydrogenase catalyzed t h e oxidation of ethanol. By recycling one of the products of the reaction, it was possible to displace the equilibrium and favor the production of acetaldehyde. The flow-through electrode was made of graphite felt and had a specific area of 275 cm-'. A mathematical model taking into account the enzymatic and electrochemical reaction rates as well as the mass transfer to the electrode was used to analyze the results. The limiting steps in the reactor are the electrochemical reaction for low potentials and the cofactor mass transfer for high potentials.