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Direct minimization in mc scf theory. the quasi-newton method

✍ Scribed by Richard H.A. Eade; Michael A. Robb


Publisher
Elsevier Science
Year
1981
Tongue
English
Weight
532 KB
Volume
83
Category
Article
ISSN
0009-2614

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✦ Synopsis


The efficiency of the use of a diagonal approximation to the hessian matrix coupled with a quasi-Newton updating method in MC SCF calculations is examined. In general, satisfactory convergence is obtained provided the CI expansion corresponds to a full valence shell CL