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Diffusion in surface-wetting films in a two-phase saturated porous solid characterised by pulsed magnetic field gradient NMR

✍ Scribed by William M. Holmes; Robin G. Graham; Ken J. Packer


Publisher
Elsevier Science
Year
2001
Tongue
English
Weight
168 KB
Volume
83
Category
Article
ISSN
1385-8947

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✦ Synopsis


Pulsed-field-gradient NMR measurements of the one-dimensional probability-density distribution P ∆ (X) for diffusive displacements of water molecules in times ∆ in a water-wet sandstone, saturated with a mixture of dodecane and brine, are presented for water saturations S w ≤ 0.32. The distributions show a distinctive shape which is attributed to the distribution of the aqueous phase in thin, locally curved and effectively two-dimensional layers on the pore surface. The data are reproduced well by a simple model in which diffusion is restricted to the surfaces of an isotropic array of infinite planes, with an effective diffusion coefficient D 2 (∆) which shows a systematic dependence on ∆. This is suggested to arise, in the main, from local curvature of the pore surface.