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Determination of selenium speciation in river waters by adsorption on iron(III)-Chelex-100 resin and differential pulse cathodic stripping voltammetry

✍ Scribed by Tommaso Ferri; Paola Sangiorgio


Publisher
Elsevier Science
Year
1996
Tongue
English
Weight
679 KB
Volume
321
Category
Article
ISSN
0003-2670

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✦ Synopsis


This paper des~hes the preconcentration of Se(IV) from peHuted waters by irun(IH)-loaded Chelex-100 resin and its determination by differential pulse cathodic stripping voltammetry. The method is used to study selenium speciatm in waters, and a speciation method, suitable for concentratinn levels of environmental significance (ng/I), is defined and applied to a real polluted system (Tevere river). Besides the determination of Se(IV) and Se(VI), the method allows discrimination between "free" and "bound" dissolved Se(IV). As regards bound Se(IV), a non.labile interaction with an "unidentified species" is hypothesised and the conditional formation constant of the hypothesised process evaluated as well as the concentration of "unidentified species". Finally, the distn'bution of Se(VI) and -(IV) added to untreated water samples was studied.