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Dass Hydrierprodukt eines β-Nitro-N-nitrosoamins ist kein 1,2,3-Triazolidin, sondern ein β-Hydroxylamino-N-nitrosoamin

✍ Scribed by Notker Egger; Lienhard Hoesch; André S. Dreiding


Book ID
102252409
Publisher
John Wiley and Sons
Year
1982
Tongue
German
Weight
344 KB
Volume
65
Category
Article
ISSN
0018-019X

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✦ Synopsis


The Product of Hydrogenation of a β‐Nitro‐N‐nitrosoamine Is Not a 1,2,3‐Triazolidine, but a β‐Hydroxylamino‐N‐nitrosoamine

It is shown, by spectroscopy, that the product of catalytic hydrogenation of N, 2‐dimethyl‐2‐nitro‐N‐nitrosopropylamine (1) consists of a 5:1 mixture of (E)‐ and (Z)‐2‐hydroxylamino‐N, 2‐dimethyl‐N‐nitrosopropylarnine (3) and does not contain ‐ as had been claimed ‐ any l, 2‐dihydroxy‐1, 2, 3‐triazolidine (2). Thus there is still no evidence for the existence of the N(OH)N(OH) functionality. The structure of intermediates on the way to 1 are also revised.