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Crystal structure of anhydrous hexakis-(2,3,6-tri-O-methyl)-cyclomaltohexaose (permethyl-α-cyclodextrin) grown from hot water and from cold NaCl solutions

✍ Scribed by Thomas Steiner; Wolfram Saenger


Publisher
Elsevier Science
Year
1996
Tongue
English
Weight
559 KB
Volume
282
Category
Article
ISSN
0008-6215

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✦ Synopsis


An X-ray diffraction study was carried out on anhydrous permethyl-a-cyclodextrin crystallized from aq solution at 40 °C, space group P212121 with a = 15.424(9), b = 18.167(7), c = 23.128(8) ,~, vol = 6481(5) ~3. The molecule is boat-shaped with the narrow end of the cyclodextrin cavity closed by two diametrically opposing glucose residues. These are strongly tilted towards the molecular axis, so that their primary methoxy groups form van der Waals contacts across the molecular opening. The remaining cavity volume is occupied by the methoxy group of a neighboring molecule (self-inclusion). From solutions containing 1 M NaCl, anhydrous permethyla-cyclodextrin crystallizes isomorphously at room temperature.