Creation of spin coherent states in the course of chemical reactions
β Scribed by Kev M. Salikhov
- Publisher
- Elsevier Science
- Year
- 1993
- Tongue
- English
- Weight
- 320 KB
- Volume
- 201
- Category
- Article
- ISSN
- 0009-2614
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β¦ Synopsis
In many elementary chemical acts, electron and nuclear spins can be found in coherent states. The necessary conditions are formulated for formation of coherent spin states in the course of chemical reactions. Some possible experimental manifestations of chemically induced coherent spin states are discussed.
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## Rcceivcd 21 Jl?ly 1975 We present a theoretical model for describing spin coherence in photoexcited triplet states in zero-field under the influence of vibronic relaxation. From a comparison with experimental results in parabenzoquinone we obtain information about the properties of the excited