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Coupled perturbation theory within the antisymmetrized product of separated geminals (APSG) framework

✍ Scribed by Yu. Dmitriev; G. Peinel


Publisher
John Wiley and Sons
Year
1981
Tongue
English
Weight
319 KB
Volume
19
Category
Article
ISSN
0020-7608

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✦ Synopsis


Abstract

A coupled perturbation theory for the antisymmetrized product of separated geminals (APSG) approximation is derived. The variational principle for the APSG wave function in an external oscillating field is employed and a set of equations of the form analogous to the normal RPA is obtained. At this level the reduced resolvent in the form of a spectral expansion is written and it is used for the evaluation of the second‐order properties.