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Counterpoise corrected calculations at the correlated level: A simplified method using LMOs

✍ Scribed by C. Kozmutza; E. Kapuy


Publisher
John Wiley and Sons
Year
1991
Tongue
English
Weight
660 KB
Volume
12
Category
Article
ISSN
0192-8651

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✦ Synopsis


Ab initio calculations have been performed in order to investigate the counterpoise corrections, especially at the correlated level for molecular interactions. It is pointed out that, when using a localized representation, the calculations using the MBPT/MPB method can be simplified. The H,O + H,O system was studied, with the use of 6-31 G* basis set. The method allows one to determine the intramolecular correlation components in a simplified way. Boys' localization procedure was applied throughout, both in the occupied as well as in the virtual spaces.