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Controlled Fluorescence Bursts from Conjugated Polymers Induced by Triplet Quenching

✍ Scribed by F. Schindler; J. M. Lupton; J. Feldmann; U. Scherf


Publisher
John Wiley and Sons
Year
2004
Tongue
English
Weight
127 KB
Volume
16
Category
Article
ISSN
0935-9648

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✦ Synopsis


Dramatic fluorescence bursts (see Figure and cover) from conjugated polymers are observed upon exposure to air. The burst occurs prior to photo‐oxidation and is imaged in single molecules of a ladder‐type polymer, but is also found in bulk films. Triplet shelving is identified as an important mechanism limiting the fluorescence yield of conjugated polymers due to both a reduction in photon cycling rates and singlet–triplet quenching in the multichromophoric system.