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Control of the CT interaction between electron-donor and -acceptor moieties of a 1,4-dicyanonaphthalene–arene dyad for intermolecular exciplex or excimer formation in crystals

✍ Scribed by Mitsutaka Imoto; Hiroshi Ikeda; Maki Ohashi; Motonori Takeda; Akihiro Tamaki; Hisaji Taniguchi; Kazuhiko Mizuno


Publisher
Elsevier Science
Year
2010
Tongue
French
Weight
681 KB
Volume
51
Category
Article
ISSN
0040-4039

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✦ Synopsis


Colorless crystals of 1,4-dicyano-2-(4 0 -methoxybenzyloxy)methylnaphthalene (2), which is a 1,4-dicyano-2-methylnaphthalene (DCMN)-4-methylanisole (MA) dyad linked by an ether unit, selectively form a fluorescent intermolecular DCMN-MA exciplex (greenish blue, k exciplex f ¼ 456 nm). In contrast, 1,4-dicyano-2-(4 0 -methylbenzyloxy)methylnaphthalene (3), which is a DCMN-p-xylene dyad, forms a fluorescent intermolecular DCMN-DCMN excimer in the crystalline state (blue, k excimer f