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Control of Diastereo- and Enantioselectivity in Metal-Catalyzed 1,3-Dipolar Cycloaddition Reactions of Nitrones with Alkenes. Experimental and Theoretical Investigations

✍ Scribed by Gothelf, Kurt V.; Hazell, Rita G.; Jørgensen, Karl Anker

Book ID
120305208
Publisher
American Chemical Society
Year
1996
Tongue
English
Weight
351 KB
Volume
61
Category
Article
ISSN
0022-3263

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✍ Kim B. Jensen; Kurt V. Gothelf; Karl Anker Jørgensen 📂 Article 📅 1997 🏛 John Wiley and Sons 🌐 German ⚖ 529 KB

Catalytic control of regio-, diastereo-, and enantioselectivity in the 1,3-dipolar cycloaddition of 3-acryloyloxazolidin-2-one (4) with different nitrones 2 by the application of a [TiX,(TADDOLato)] complex as the catalyst was developed (TADDOL = a,ru,a',a'-tetraary1-1,3-dioxolane-4,5-dimethanol). I