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Control by density effects of the Rydberg-valence configuration mixing in matrix isolated NO

✍ Scribed by M. Chergui; R. Reininger; E. Morikawa; A. Tramer


Publisher
Elsevier Science
Year
1993
Tongue
English
Weight
679 KB
Volume
216
Category
Article
ISSN
0009-2614

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✦ Synopsis


Density effects and Ns co-doping of Kr solids doped with NO allow continuous tuning of the NO Rydberg state energies in a range 0.35 to 0.68 eV blue of the gas phase. This property is exploited to control the vibronic contiguration mixing between the Rydberg C *II and the valence B *lI states. The influence on the interference lineshapes resulting from the interaction of discrete valence bands with the broad multiphonon Rydberg bands is discussed in terms of estimates of the Fano indices.