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Contracted and supercontracted basis sets in the theoretical treatment of coordination compounds: The cyclopentadienyl anion and ferrocene

✍ Scribed by Renzo Cimiraglia; Daniel Maynau; Maurizio Persico


Publisher
Elsevier Science
Year
1988
Tongue
English
Weight
317 KB
Volume
153
Category
Article
ISSN
0009-2614

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✦ Synopsis


In this paper we apply a technique, recently proposed for organic substituents, to the cyclopentadienyl anion. The technique allows us to reduce the size of the basis set without seriously affecting the quality of the ab initio calculations. This is illustrated by the determination of the Fe-ring distance in ferrocene, which is known to require a high level ab initio treatment including electron correlation.