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Conformational properties of cyclic pentaalkoxy phosphoranes: Apical–equatorial attachment and nonchair conformation of the phosphorus-containing six-membered ring

✍ Scribed by Jaehoon Yu; Alan E. Sopchik; Atta M. Arif; Wesley G. Bentrude; G.-V. Roeschenthaler


Publisher
John Wiley and Sons
Year
1991
Tongue
English
Weight
649 KB
Volume
2
Category
Article
ISSN
1042-7163

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✦ Synopsis


A series of' phosphoranes with pentacovalent phosphorus contained in a I ,3,2-dioxaphosphorinane ring have been studied by ' H Nh4R. One compound was investigated by low-temperature'3C N M R and another by X-ray crystallography. Although the ' H N M R parameters observed are time-averaged, the coupling constants can be accounted for if the phosphoranes have the six-membered ring attached apicalequatorial to phosphorus and occupy in solution rapidly isomerizing boat or slightly twisted boat conformations similar to that found in the X-ray study.