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Conformational energy minimization by simulated annealing using molecular dynamics: Some improvements to the monitoring procedure

✍ Scribed by F. Lelj; P. Grimaldi; P. L. Cristinziano


Publisher
Wiley (John Wiley & Sons)
Year
1991
Tongue
English
Weight
547 KB
Volume
31
Category
Article
ISSN
0006-3525

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✦ Synopsis


The possibility of using molecular dynamics techniques as a tool for simulated annealing is tested in the case of the molecule of biological interest N-acetyl, "-methyl amides of 3 (S) -hydroxy, 4 ( S ) -amino 6-methyl heptanoic acid [ (3S,4S) -statinel and of its (3R,4S) diastereomer. The approach is able to reach global minimum in the conformational space in the case of the mentioned molecule. A description of the method is given. The use of fractional fluctuations of the internal potential energy as an indicator able to point out transition from a given minimum region to a deeper one is investigated. The results about the lowest energy conformation of (3S,4S) diastereomer are in fairly good accordance with the results obtained in the case of search within the whole conformational hyperspace.