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Computer simulation of cage processes and some difficulties with present models

✍ Scribed by Cheves Walling; Arthur R. Lepley

Publisher
John Wiley and Sons
Year
1971
Tongue
English
Weight
368 KB
Volume
3
Category
Article
ISSN
0538-8066

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✦ Synopsis

Abstract

A simple model involving random displacements of particles in a cubic lattice is used to evaluate the importance of primary and secondary recombination in cage processes and leads to estimates of the lifetime of cage pehnomena. However, it is pointed out that all such models, and treatments which attempt to relate processes at the molecular level with bulk viscosity or diffusion constants, are inherently qualitative since they ignore the important correlation between motions of neighboring molecules.

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