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Complexation of hydroxylated ent-kaurane diterpenoids with boric acid as an aid to the assignment of the 13C NMR spectra

✍ Scribed by Francisco Fernández-Gadea; María L. Jimeno; Benjamín Rodríguez


Publisher
John Wiley and Sons
Year
1984
Tongue
English
Weight
552 KB
Volume
22
Category
Article
ISSN
0749-1581

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✦ Synopsis


The 13C NMR spectra of some hydmxylated e n t -k a m e diterpenoids were measured in CDC13-Py-4 (1 : 1) solutiou and also after addition of boric acid. Complexation of ent-3P,l8-, ent-7a;15&, ent-7a,l5cu-, ent-l5B,16B-and ent-16B,17-dihydroq derivatives with boric acid produced considerable chemical shift changes and marked broadening of the signals of the hydroxy-bearing and neighbouring carbon atoms. This behaviour provides a useful and reliable method for assigning the '"C NMR spectra of these compounds.