𝔖 Bobbio Scriptorium
✦   LIBER   ✦

Complete large-molecule high-resolution mass spectra from 50-femtomole microvolume injection

✍ Scribed by Neil L. Kelleher; Michael W. Senko; Daniel P. Little; Peter B. O'Connor; Fred W. McLafferty


Book ID
103996792
Publisher
Elsevier Science
Year
1995
Tongue
English
Weight
183 KB
Volume
6
Category
Article
ISSN
1044-0305

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✦ Synopsis


For electrospray ionization in Fourier-transform mass spectrometry, direct injection of 5×10(-14) mol (0.5 µL of 100 nM from a microvolume sample valve) of ubiquitin (8565 Da) into the flowing solvent stream yields a spectrum with 85:1 signal-to-noise ratio, 2-ppm mass accuracy, and isotopic resolution. Gated trapping for 100 µs from a 0.15-µL/min injection of 20-µM ubiquitin consumes 5×10(-18) mol, which produces a spectrum with 23:1 signal-to-noise ratio and τ;3×10(5) resolving power.