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Comparison of perturbatively corrected MRD CI results with a full CI treatment of the BH ground state

✍ Scribed by Peter G. Burton; Robert J. Buenker; Pablo J. Bruna; Sigrid D. Peyerimhoff


Publisher
Elsevier Science
Year
1983
Tongue
English
Weight
681 KB
Volume
95
Category
Article
ISSN
0009-2614

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✦ Synopsis


It is demonstrated by direct comparison with a full CI calculation for BH (DZ basis at re) that the corresponding energy value can be obtained to hi@ accuracy (0.01 kJ/mol-l) by employins cstrapolation from a series of MRD CI trurments which consider at most a small fraction of the total configuration space (order I7019 versus 132686). The perturbative methods employed L&T of quite general applicability and are seen to provide high ovenlI accuracy in an economically fcaslble manner. Volume 95. numhcr 4.5 CHEMICAL PHYSICS LFD-TERS