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Comparison of HPLC and CZE methods for analysis of DOTA-like esters – reaction intermediates in synthesis of magnetic resonance contrast agents

✍ Scribed by Anna Hamplová; Tomáš Křížek; Vojtěch Kubíček; Zuzana Bosáková; Pavel Coufal


Publisher
John Wiley and Sons
Year
2010
Tongue
English
Weight
192 KB
Volume
33
Category
Article
ISSN
1615-9306

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✦ Synopsis


Abstract

RP‐HPLC and non‐aqueous CZE methods were evaluated for qualitative and quantitative analysis of esterified macrocyclic compounds of the DOTA family (DOTA=1,4,7,10‐tetraazacyclododecan‐1,4,7,10‐tetraacetic acid). This group of compounds represents important reaction intermediates in synthesis of magnetic resonance contrast agents. Calibration curves in the concentration range from 1.0×10^−5^ to 1.0×10^−3^ mol/L were plotted and the experimental data were critically compared in terms of their repeatability, linearity, LOD and LOQ. The optimized methods were successfully applied to the analysis of a real reaction mixture without any further pretreatment.