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Collisionless vibrational energy redistribution between infrared and Raman active modes in SF6

✍ Scribed by E. Mazur; I. Burak; N. Bloembergen

Publisher: Elsevier Science
Year: 1984
Tongue: English
Weight: 385 KB
Volume: 105
Category: Article
ISSN: 0009-2614
DOI: 10.1016/0009-2614(84)85025-3

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✦ Synopsis

Fiperimental results fiom a tiene-icsolvad Raman study of collisionless ( (p_{\text {meve }}<0.05) ns rort: mobs (<2) ns Tom) infrired multiphoton evcited SF; ase reported Fiven at ufrared fluenors behw (011 / \mathrm{cm}^{2}) intiamolecular eneri:y redistsibution is obsetved. Comparison with photoacoustic ineosure ments shows that within experimental acceracy these is equipastilioning among the vilsous vibrational modes

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Vibrational energy relaxation and vibrational cooling of polyatomic liquids were studied with the ultrafast infrared-Raman (IR-Raman) technique. In the IR-Raman technique, a type of two-dimensional vibrational spectroscopy, a vibrational transition is pumped with a mid-infrared pulse and the instant