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Collisional narrowing and spectral shift in coherent anti-stokes Raman spectra of molecular nitrogen up to 2500 bar and 700 K

✍ Scribed by Th. Bouché; Th. Dreier; B. Lange; J. Wolfrum; E. U. Franck; W. Schilling


Book ID
104761790
Publisher
Springer
Year
1990
Tongue
English
Weight
668 KB
Volume
50
Category
Article
ISSN
0721-7269

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✦ Synopsis


CARS spectra of the N 2 Q-branch up to 2500 bar and 700 K have been measured. Calculated spectra based on theoretical models show significant disagreement with measured spectra above 300 bar so that CARS temperature measurements are in error by 130 K at 700 K and -150 K at 295 K. The spectral shift of the Q-branch reaches an asymptotic value corresponding to that measured in liquid nitrogen.