Coherent spin radiation by magnetic nanomolecules and nanoclusters

✍ Scribed by V.I. Yukalov; V.K. Henner; P.V. Kharebov; E.P. Yukalova

• Publisher: John Wiley and Sons
• Year: 2008
• Tongue: English
• Weight: 257 KB
• Volume: 5
• Category: Article
• ISSN: 1612-2011
• DOI: 10.1002/lapl.200810077

✦ Synopsis

The peculiarities of coherent spin radiation by magnetic nanomolecules is investigated by means of numerical simulation. The consideration is based on a microscopic Hamiltonian taking into account realistic dipole interactions. Superradiance can be realized only when the molecular sample is coupled to a resonant electric circuit. The feedback mechanism allows for the achievement of a fast spin reversal time and large radiation intensity. The influence on the level of radiation, caused by sample shape and orientation, is analysed. The most powerful coherent radiation is found to occur for an elongated sample directed along the resonator magnetic field. s(t) -0.5 0 0.5 1.0 -1.0 1.00 0.75 0.50 0.25 0 t Reduced spin polarization s(t) as a function of dimensionless time for N = 144 molecules of spin S = 10, with ω 0 = 2000, ωD = 20, and γ = 30, for different sample shapes and orientations: the chain of spins along the z-axis (solid line), the chain along the x-axis (long-dashed line), the yz plane of spins (short-dashed line), and the xy plane of spins (dotted-dashed line)