✦ LIBER ✦

Coherent raman spectroscopy of HCN complexes

✍ Scribed by G.A. Hopkins; M. Maroncelli; J.W. Nibler; T.R. Dyke

Publisher: Elsevier Science
Year: 1985
Tongue: English
Weight: 511 KB
Volume: 114
Category: Article
ISSN: 0009-2614
DOI: 10.1016/0009-2614(85)85063-6

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✦ Synopsis

Photoacoustic

Raman spectroscopy (PARS) is shown to be a sensitive technique for obtaining Raman spectra of hydrogenbonded complexes io the gas phase. Coherent anti-Stokes Raman spectroscopy (CARS) prondes analogous spectra in supersonic expansions. The effective resolution is higher in the latter QSP-due to the cooling and collision-free condi-t~ons in thelet. The ability to "tune" complex size by changing expansion conditions is demonstrated in the case of HCN.

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