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Coherent anti-stokes raman scattering in gaseous nitrogen with picosecond pulses

✍ Scribed by B.I. Greene; R.B. Weisman; R.M. Hochstrasser

Publisher
Elsevier Science
Year
1978
Tongue
English
Weight
428 KB
Volume
59
Category
Article
ISSN
0009-2614

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✦ Synopsis

The use of CARS as a probe of gas phase molecular concentrations has been extended into the picosecond regime. A double-beam configuration employing singe pulses from a mode-locked Nd:glass laser has allowed measurement of Nz ('Q, u = 0) pressures to an accuracy of better than 10% with 8 ps time resolution. This technique shows promise for the study of dy%unics of gas phase photodissociation processes

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