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Cluster model of glass transition. The variation of Tg with cage vibrational frequency of Na+ ions in sodium borovanadate glasses

✍ Scribed by S. Muthupari; K.J. Rao


Book ID
103035630
Publisher
Elsevier Science
Year
1994
Tongue
English
Weight
473 KB
Volume
223
Category
Article
ISSN
0009-2614

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✦ Synopsis


The cage vibrational frequencies of Na+ ions in sodium borovanadate glasses have been examined using far-infrared spectroscopy. The glass transition temperature, T,, is found to vary linearly with the cage vibrational frequency, v. The variation of v has been related to the average excess partial charge on the cage oxygen atoms and hence to the force constant. The observed linear variation of T, as a function of v has been rationalized on the basis of the cluster model of glass transition.