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Cleavage of an Ether Bond via β-Elimination of Ethanol from [(H2O)5CrCH2CH2OC2H5]2+ in Aqueous Solutions; A Pulse Radiolysis Study

✍ Scribed by Dr. Haim Cohen; Prof. Dr. Dan Meyerstein


Publisher
John Wiley and Sons
Year
1985
Tongue
English
Weight
325 KB
Volume
24
Category
Article
ISSN
0044-8249

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✦ Synopsis


temperature range 100-298 K were readily fitted using an isotropic Heisenberg model, H'= 2 J S , .Sz ( S , =Sz = 2) and g = 2.24. The spin exchange coupling constant J of -14(2) cm -I," 'I which is in excellent agreement with the value derived for deoxyhemerythrin,[61 indicates weak antiferromagnetic behavior. 1 is thus a very good model for the bonding of the Fe" centers in deoxyhemerythrin and confirms the structure proposed by Solomon et a1.161 and Stenkamp et al.["l 600 800 1000 1200 400 L90 580 670 760 850 h(nm] -X[nm]

[I] a) R.