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Chirality transmission via tandem sigmatropic rearrangement: Regio- and stereochemical outcome in the tandem Wittig—oxy-Cope sequence of allyl cis-5-methyl-2-cyclohexenyl ether

✍ Scribed by Noboru Sayo; Yasuhiro Kimura; Takeshi Nakai


Book ID
104221187
Publisher
Elsevier Science
Year
1982
Tongue
French
Weight
238 KB
Volume
23
Category
Article
ISSN
0040-4039

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✦ Synopsis


The tztled szgmatropzc sequence proceeds wzth compZete net retentzon of confzguratzon, and surprzszngly, suffers from a regzochemzcal compZccat-z,on arzstng maznly from the unexpected competztzon of the i2,37-vs. L-1,23-shzft zn the Wzttzg process, as reveaZed by the use of the deuterzwn-labeled substrate