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Chiral synthesis via organoboranes. 25. B-(Z and E)-crotylbis-(2-isocaranyl)boranes as valuable reagents for the asymmetric crotylboration of aldehydes

✍ Scribed by Herbert C. Brown; Ramnarayan S. Randad


Publisher
Elsevier Science
Year
1990
Tongue
French
Weight
351 KB
Volume
46
Category
Article
ISSN
0040-4020

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✦ Synopsis


The asymmetric crotylboration of representative aldehydes, RCHO (R = Me, Et-), with B-[Z and El-crotylbis@isocaranyl)boranes (4 and 5) proceeds with remarkably high enantioselectivity (>94-98% ee) and diastereoselectivity (>99% de) at -78 Oc in ethyl ether.