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Chemistry in Environmentally Benign Media, 8 Hydroxymethyl Functionalized Phosphanes as Building Blocks to new Water-Soluble Gold(I) Complexes - synthesis, Characterization, and X-ray crystal Structures of Novel Tetrahedral [Au{P(CH2OH)3}4]+ and Trigonal Planar [Au(Ph2PCH2OH)3]+ Gold (I) Complexes

✍ Scribed by Berning, Douglas E. ;Katti, Kattesh V. ;Barnes, Charles L. ;Volkert, Wynn A.


Publisher
Wiley (John Wiley & Sons)
Year
1997
Tongue
English
Weight
473 KB
Volume
130
Category
Article
ISSN
0009-2940

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✦ Synopsis


The reactions of water-soluble phosphanes P(CH,OH), (1) and Ph2PCH20H (2) with NaAuC14 in aqueous or alcoholic media, produced the water/alcoholic-soluble Au' complexes [Au(P(CH,OH),),]+ (3) and [Au(Ph2PCH20H):J+ (4) in near quantitative yields. The X-ray structures of 3 and 4, reported in this paper, confirm the structures of these new generation of water-soluble transition metal complexes. All compounds were characterized by 'H-, 13C-, "P-NMR spectroscopy and mass spectrometry. The structures of 3 and 4 were determined by X-ray crystallography.