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ChemInform Abstract: ZrCl4-Mediated Regioselective Electrophilic Amination of Activated Arenes with New Alkyl Arylaminocarbonyldiazenecarboxylates: Intermolecular and Intramolecular Reactions.

✍ Scribed by Roman Lenarsic; Marijan Kocevar; Slovenko Polanc


Publisher
John Wiley and Sons
Year
2010
Weight
37 KB
Volume
30
Category
Article
ISSN
0931-7597

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✦ Synopsis


The title diazenes are found to be new and convenient reagents for the regioselective electrophilic amination of various electron-rich arenes.

The products serve as potent precursors of arylsubstituted hydrazines, ureas, and 1,2,4-triazolinediones. In the absence of activated arenes the diazenes undergo intramolecular cyclization, providing a simple route to benzimidazoles of type (VI). -(LENARSIC,