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ChemInform Abstract: Synthesis of Wasabidienone A via a Novel Acyl Rearrangement Reaction from Carbon to Oxygen.

✍ Scribed by S. SATO; H. OBARA; K. YUSA; K. SUDO; M. SANDO; H. KAGAYA; H. IJICHI; S. MATSUBA; T. KAMAZAWA; J. ONODERA

Publisher
John Wiley and Sons
Year
2010
Weight
38 KB
Volume
29
Category
Article
ISSN
0931-7597

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✦ Synopsis

Synthesis of Wasabidienone A via a Novel Acyl Rearrangement

Reaction from Carbon to Oxygen.

-The key step in the synthesis of the yellow pigment wasabidienone A (VII) is the rearrangement of an acyl group from carbon to the Ξ²-hydroxy oxygen of the cyclohexadienone (V). This novel type of reaction is extended to other cyclohexadienones [cf. (VIII), 10 examples] with low to excellent result. -(

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