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ChemInform Abstract: Reaction of H2 and H2S with CoMoO4 and NiMoO4: TPR, XANES, Time-Resolved XRD, and Molecular-Orbital Studies.

✍ Scribed by Jose A. Rodriguez; Sanjay Chaturvedi; Jonathan C. Hanson; Joaquin L. Brito

Publisher: John Wiley and Sons
Year: 2010
Weight: 34 KB
Volume: 30
Category: Article
ISSN: 0931-7597
DOI: 10.1002/chin.199920010

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✦ Synopsis

Reaction of H 2 and H 2 S with CoMoO 4 and NiMoO 4 : TPR, XANES, Time-Resolved XRD, and Molecular-Orbital Studies.

-The reactivity of a series of metal molybdates (α-MMoO 4 , β-MMoO 4 , MMoO 4 •nH 2 O, M: Co, Ni) toward H 2 and H 2 S is examined using temperature programmed reduction, X-ray methods and ab initio calculations. In general, these molybdates are more reactive toward H 2 and easier to reduce than pure molybdenum oxides. Moreover, the molybdates interact stronger with H 2 S than MoO 3 or MoO 2 . Reoxidation of the reduced and sulfided molybdates is achieved by reaction with O 2 at high temperatures. -(RODRIGUEZ, JOSE A.; CHATURVEDI,

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