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ChemInform Abstract: Novel Palladium-Catalyzed Formal [3 + 2] Cycloaddition via Hydrocarbonation Reactions of Allenes.

✍ Scribed by Masaki Meguro; Yoshinori Yamamoto

Publisher
John Wiley and Sons
Year
2010
Weight
33 KB
Volume
30
Category
Article
ISSN
0931-7597

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✦ Synopsis

Novel Palladium-Catalyzed Formal [3 + 2] Cycloaddition via Hydrocarbonation Reactions of Allenes.

-The palladium-catalyzed reaction of activated olefins (I), (IV), (VI), and (VIII) with allenes (II) and (Xa), bearing an activated methine at the carbon chain terminus, gives cyclopentanes with good to excellent yields. The present cycloaddition reaction provides an entirely new procedure for constructing cyclopentanoids under neutral conditions. -

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