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ChemInform Abstract: Ni-Catalyzed Cross Coupling of Alkoxide-Containing Vinyl Halides with Grignard Reagents. A “One-Pot” Synthesis of 2-((Trimethylsilyl)methyl)- 2-propen-1-yl Acetate.

✍ Scribed by M. G. ORGAN; A. P. MURRAY


Publisher
John Wiley and Sons
Year
2010
Weight
32 KB
Volume
28
Category
Article
ISSN
0931-7597

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✦ Synopsis


Ni-Catalyzed Cross Coupling of Alkoxide-Containing Vinyl

Halides with Grignard Reagents.

A "One-Pot" Synthesis of 2-((Trimethylsilyl)methyl)-2-propen-1-yl Acetate.

-A convenient and general one-pot strategy for the title reaction is developed and applied to the synthesis of title compound (IX) which is a useful trimethylene methane precursor. Vinyl iodides, e.g. (VIb), are not suitable for this reaction due to halogen-metal exchange prior to the coupling step. -(ORGAN, M. G.;