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ChemInform Abstract: Homogeneous Catalytic Dimerization of Terminal Alkynes by C5Me5Ru(L)H3 (L: PPh3, PCy3, PMe3) (I).

✍ Scribed by C. S. YI; N. LIU


Publisher
John Wiley and Sons
Year
2010
Weight
32 KB
Volume
28
Category
Article
ISSN
0931-7597

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✦ Synopsis


Homogeneous Catalytic Dimerization of Terminal Alkynes by C5Me5Ru(L)H3 (L: PPh3, PCy3, PMe3) (I).

-Selective product formation of (III), (IV), and/or (V) in the title reaction is effected by modulating both catalyst environment and the alkyne substrate. Cumulene (VI), a rare form of dimer, is cleanly obtained from (IIe). A mechanistic interpretation is given based on the product distribution. -(YI, C.