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ChemInform Abstract: Chelation-Assisted RhI-Catalyzed ortho-Alkylation of Aromatic Ketimines or Ketones with Olefins.

✍ Scribed by Chul-Ho Jun; Choong Woon Moon; Jun-Bae Hong; Sung-Gon Lim; Kwan-Yong Chung; Yeon-Hee Kim

Publisher: John Wiley and Sons
Year: 2010
Weight: 34 KB
Volume: 33
Category: Article
ISSN: 0931-7597
DOI: 10.1002/chin.200227068

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Described herein is the Rh I -catalyzed ortho-alkylation of aromatic ketimines or ketones with olefins. This method showed high reactivity and selectivity to monoalkylation for a variety of olefins including 1-alkenes with an allylic proton, a,w-dienes, and internal olefins. For a mechanistic study,

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