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ChemInform Abstract: Carbocyclic cis-(1.1.1)-Tris-σ-homobenzenes - Syntheses by Triple Epoxide → Cyclopropane Conversions, Structural Data, (. sigma.2s + σ2s + σ2s) Cycloreversions.

✍ Scribed by C. RUECKER; H. MUELLER-BOETTICHER; W.-D. BRASCHWITZ; H. PRINZBACH; U. REIFENSTAHL; H. IRNGARTINGER


Publisher
John Wiley and Sons
Year
2010
Weight
33 KB
Volume
28
Category
Article
ISSN
0931-7597

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✦ Synopsis


Carbocyclic cis-(1.1.1)-Tris-σ-homobenzenes -Syntheses by Triple Epoxide → Cyclopropane Conversions, Structural Data, (. sigma.2s + σ2s + σ2s) Cycloreversions.

-A weakly basic mixed cyanocuprate carbon nucleophile is the reagent of choice to open the triple epoxide (I) to fully substituted cyclohexane derivatives such as (II), which in several group manipulations can be transformed into cyclopropane derivatives such as (III).