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ChemInform Abstract: Biomimetic Reductive Amination of Fluoro Aldehydes and Ketones via (1, 3)-Proton Shift Reaction. Scope and Limitations.

✍ Scribed by T. ONO; V. P. KUKHAR; V. A. SOLOSHONOK


Publisher
John Wiley and Sons
Year
2010
Weight
33 KB
Volume
28
Category
Article
ISSN
0931-7597

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✦ Synopsis


Biomimetic Reductive Amination of Fluoro Aldehydes and Ketones via (1, 3)-Proton Shift Reaction. Scope and Limitations.

-Azomethine-azomethine isomerization of the fluorinated Schiff's bases ( III) and (IX) (14 examples) affords the corresponding N-benzylidene derivatives in good yields, which can be transformed into fluorine-containing amines of potential biological interest. In the case of chlorine-and bromine-containing derivatives such as (IIIe), (IIIf) and (XII), additional dehydrohalogenation takes place. -