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ChemInform Abstract: Asymmetric Quadruple Aminocatalytic Domino Reactions to Fused Carbocycles Incorporating a Spirooxindole Motif.

✍ Scribed by Kun Jiang; Zhi-Jun Jia; Xiang Yin; Li Wu; Ying-Chun Chen


Publisher
John Wiley and Sons
Year
2010
Weight
66 KB
Volume
41
Category
Article
ISSN
0931-7597

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✦ Synopsis


Abstract

A three‐component, domino Michael—Michael—Michael—aldol process of the indole‐derived substrates of the type (I) with two identical or different molecules of α,β‐unsaturated aldehydes under quadruple iminium/enamine/iminium/enamine catalysis affords a variety of the enantiomerically pure hydroindane derivatives, bearing six contiguous stereocenters and a spirooxindole motif with complete diastereoselectivities [cf.