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ChemInform Abstract: A Highly Efficient Synthesis of (-)-PI-091 Construction of the 4- Alkoxy-2-butene-4-lactam Skeleton from Fischer-Type Carbene Complexes, Alkynyllithiums, and Tosyl Isocyanate.

✍ Scribed by N. IWASAWA; K. MAEYAMA


Publisher
John Wiley and Sons
Year
2010
Weight
35 KB
Volume
28
Category
Article
ISSN
0931-7597

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✦ Synopsis


A Highly Efficient Synthesis of (-)-PI-091 Construction of the 4-Alkoxy-2-butene-4-lactam Skeleton from Fischer-Type Carbene Complexes, Alkynyllithiums, and Tosyl Isocyanate.

-A general and facile method for the construction of lactams such as ( IV) is developed by the reaction of the propargyl metallic species, generated from Fischer-type carbene complexes and alkynyllithiums, and tosyl isocyanate. Starting from (Ia) and (V) this approach is applied to an enantioselective synthesis of the title product (X). -(IWASAWA, N.;